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Bioaccumulation of Per- and polyfluoroalkyl substances (PFASs) in a tropical estuarine food web
IVL Swedish Environmental Research Institute.
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2020 (English)In: Science of the Total Environment, ISSN 0048-9697, E-ISSN 1879-1026Article in journal (Refereed) Published
Abstract [en]

Abstract The biomagnification of per- and polyfluoroalkyl substances (PFASs) was investigated in a tropical mangrove food web from an estuary in Bahia, Brazil. Samples of 44 organisms (21 taxa), along with biofilm, leaves, sediment and suspended particulate matter were analyzed. Sum (∑) PFAS concentrations in biota samples were dominated by perfluorooctane sulfonate (PFOS, 93% detection frequency in tissues; 0.05 to 1.97 ng g⁻¹ ww whole-body (wb)), followed by perfluorotridecanoate (PFTrDA, 57%; 0.01 to 0.28 ng g⁻¹ ww wb). PFOS precursors such as perfluorooctane sulfonamide (FOSA, 54%; 0.01 to 0.32 ng g⁻¹ ww wb) and N-ethyl perfluorooctane sulfonamide (EtFOSA; 30%; 0.01 to 0.21 ng g⁻¹ ww wb) were also detected. PFAS accumulation profiles revealed different routes of exposure among bivalve, crustacean and fish groups. Statistics for left-censored data were used in order to minimize bias on trophic magnification factors (TMFs) calculations. TMFs >1 were observed for PFOS (linear + branched isomers), EtFOSA (linear + branched isomers), and perfluorononanoate (PFNA), and in all cases, dissimilar accumulation patterns were observed among different trophic positions. The apparent biodilution of some long-chain PFCAs through the food chain (TMF < 1) may be due to exposure from multiple PFAS sources. This is the first study investigating bioaccumulation of PFASs in a tropical food web and provides new insight on the behavior of this ubiquitous class of contaminants.

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2020.
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URN: urn:nbn:se:ivl:diva-3302DOI: 10.1016/j.scitotenv.2020.142146OAI: oai:DiVA.org:ivl-3302DiVA, id: diva2:1554888
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A-rapport, A2498Available from: 2021-05-17 Created: 2021-05-17

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Citation style
  • apa
  • harvard1
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
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  • de-DE
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  • en-US
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  • Other locale
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Output format
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  • asciidoc
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